A rifle barrel's harmonic frequencies are not even multiples of its resonant one.
Then they aren't harmonics. The definition of harmonics:
http://dictionary.reference.com/browse/harmonic
Physics. of, relating to, or noting a series of oscillations in which each oscillation has a frequency that is an integral multiple of the same basic frequency.
But even if they aren't harmonics, it doesn't really matter. The basic principles still apply. If you add a number of sine waves together you will always get a resulting signal which will have maxima and minima.
Search "cantilever beam vibration frequencies" then see why.
Too many folks compare rifle barrel vibration frequencies to audible frequencies from musical instruments (voices?) that "harmonize" when they are exact multiples of each other. That's different than the physics of mechanical things; rifle barrels and cantilever beams fixed at one end.
The basic principles still apply. The amplitudes of the various modes will fall off as frequency increases past the main resonant frequency and will therefore have less effect on the overall movement of the muzzle than the main resonant frequency.
another question: the shot impulse also applies 50kpsi to the breach face and the base of the bullet. would the resultant vibrations of these two impulses damp the overall vibration of the barrel? the two pulses occur simultaneous to the impulse delivered to the chamber walls, but at different locations on the barrel.
Do you have some reason to believe that they would or are you just grasping at straws? Remember a hypothesis, the first step in proving a theory or in a proper experiment, is an educated guess, not just wild speculation.
https://www.vocabulary.com/dictionary/hypothesis
A hypothesis is something more than a wild guess but less than a well-established theory.
To get an impulse to cancel would be very difficult--you could get cancellation if you input two impulses at
exactly the same point and at
exactly the same amplitudes and in
exactly opposite directions. Theoretically you could get some cancellation effect if you could very precisely control the timing/amplitude/position of an impulse input, but for two impulses to have any significant cancellation effect on each other by chance would be very unlikely.
Otherwise, making the common assumptions, the overall response will be the sum of the two impulse responses taking the input times into consideration.
...have any barrel vibration measurements been taken?
...movement of the bullet down the barrel causes the rifle to recoil (newton's third law of motion), not a vibration caused by a 50kpsi impulse.
Regardless of how the vibration is induced or what the vibration measurements show, it can be accurately represented as the sum of sine waves of differing frequencies and that the amplitudes of the various frequencies will reduce as frequency increases beyond the main resonant frequency.
We know the first part is true because of Fourier's theorem and we know the last part is true due to the physics of vibration of real-world objects.
In other words, regardless of what starts the barrel vibrating, the basic principles that make the BOSS work will still apply.