Bolt Lover;
I use that same mold and bullet and get ~2" groups at 50yds from my S&W Perf. ctr guns.
However I do the following:
1. I use aircooled w/w with ~2% added "lead-free solder" as sold at hardware/plumbing supply stores. It's 95%Tin and 5% Antimony.
2. I size to .357" with Lee push-through sizer die. Or alternatively, I use a Lyman #450 sizer/lubricator to size/lube them with SPG to .357"
3. I use 5.2gr of Hod. LongShot powder. From the 6"bbl gun these run ~1,220fps. Not HOT but not squibs either.
at the volumn of loading I do, heat-treating is too much... Not needed if diameter and alloy is correct.
I don't get much better results than you do with Bullseye or other fast burning powders (Win231, Titegroup,RedDot,WinSuperTarget,ect).
Unique, Win.SuperField, Universal, and PowerPistol have given me better 9mm results. Also, filling the lube groove with SPG is the difference between range-"burners" and match ammo.
As others stated, the 9mm can be a challenge with cast bullets.
Try posting/joining
www.cast-boolits.com